Broadband light absorption by a hemispherical concentric nanoshell array.

Achieving highly efficient broadband absorption is an important research area in nanophotonics. In this paper, a novel method is proposed to design broadband near-perfect absorbers, consisting of a four-layer hemispherical concentric nanoshell array. The proposed nanostructure supports absorptivity exceeding 95% in the entire visible region, and the absorption bandwidth is determined by the interaction or 'hybridization' of the plasmons of the inner and outer metal-based nanoshells. Moreover, the designed absorber has wide-angle capability and is insensitive to polarization. The simple structure, as well as the stable absorption properties, suggests that such core-shell nanostructures can serve as a potential candidate for many applications such as solar energy harvesting, photo-detection, and emissivity control.

Physics-guided neural network for channeled spectropolarimeter spectral reconstruction.

A reconstruction method incorporates the complete physical model into a traditional deep neural network (DNN) is proposed for channeled spectropolarimeter (CSP). Unlike traditional DNN-based methods that need to employ training datasets, the method starts from randomly initialized parameters which are constrained by the CSP physical model. It iterates through the gradient descent algorithm to obtain the estimation of the DNN parameters and then to obtain the mapping relationship. As a result, it eliminates the need for thousands of sets of ground truth data, while also leveraging the physical model to achieve high-precision reconstruction. As seen, the physical model participates in the optimization process of DNN parameters, thus achieving physical guidance for the DNN output results. Based on the characteristic of the network, we designate this method as the physics-guided neural network (PGNN). Both simulations and experiments demonstrate the superior performance of the proposed method. Our approach will further promote the practical application of CSP in a wider range of fields.

Strong coupling of multiple optical interface modes with ultra-narrow linewidth in one-dimensional topological photonic heterostructures.

Coherent coupling of optical modes with a high Q-factor underpins realization of efficient light-matter interaction with multi-channels in resonant nanostructures. Here we theoretically studied the strong longitudinal coupling of three topological photonic states (TPSs) in a one-dimensional topological photonic crystal heterostructure embedded with a graphene monolayer in the visible frequencies. It is found that the three TPSs can strongly interplay with one another in the longitudinal direction, enabling a large Rabi splitting (∼ 48 meV) in spectral response. The triple-band perfect absorption and selective longitudinal field confinement have been demonstrated, where the linewidth of hybrid modes can reach 0.2 nm with Q-factor up to 2.6 × 103. Mode hybridization of dual- and triple-TPSs were investigated by calculation of the field profiles and Hopfield coefficients of the hybrid modes. Moreover, simulation results further show that resonant frequencies of the three hybrid TPSs can be actively controlled by simply changing the incident angle or structural parameters, which are nearly polarization independent in this strong coupling system. With the multichannel, narrow-band light trapping and selectively strong field localization in this simple multilayer regime, one can envision new possibilities for developing the practical topological photonic devices for on-chip optical detection, sensing, filtering, and light-emitting.

Polarization-selective narrow band dual-toroidal-dipole resonances in a symmetry-broken dielectric tetramer metamaterial.

Here we propose a metasurface consisting of symmetry-broken dielectric tetramer arrays, which can generate polarization-selective dual-band toroidal dipole resonances (TDR) with ultra-narrow linewidth in the near-infrared region. We found, by breaking the C4v symmetry of the tetramer arrays, two narrow-band TDRs can be created with the linewidth reaching ∼ 1.5 nm. Multipolar decomposition of scattering power and electromagnetic field distribution calculations confirm the nature of TDRs. A 100% modulation depth in light absorption and selective field confinement has been demonstrated theoretically by simply changing the polarization orientation of the exciting light. Intriguingly, it is also found that absorption responses of TDRs on polarization angle follow the equation of Malus' law in this metasurface. Furthermore, the dual-band toroidal resonances are proposed to sense the birefringence of an anisotropic medium. Such polarization-tunable dual toroidal dipole resonances with ultra-narrow bandwidth offered by this structure may find potential applications in optical switching, storage, polarization detection, and light emitting devices.

Ultra-narrow-band circular dichroism by surface lattice resonances in an asymmetric dimer-on-mirror metasurface.

Narrow-linewidth circular dichroism (CD) spectroscopy is a promising candidate to push the limits of molecular handedness detection toward a monolayer or even to a single molecule level. Here, we designed a hybrid metasurface consisting of a periodic array of symmetry-breaking dielectric dimers on a gold substrate, which can generate strong CD of 0.44 with an extremely-narrow linewidth of 0.40 nm in the near-infrared. We found that two surface lattice resonance modes can be excited in the designed metasurface, which can be superimposed in the crossing spectral region, enabling a remarkable differential absorption with a high Q-factor for circular polarizations. The multipole decomposition of the resonance modes shows that the magnetic dipole component contributes most to the CD. Our simulation results also show that the CD response of the chiral structure can be engineered by modulating the structural parameters to reach the optimal CD performance. Ultra-narrow-linewidth CD response offered by the proposed metasurface with dissymmetry provides new possibilities towards design of the high-sensitive polarization detecting, chiral sensing and efficient chiral light emitting devices.

Recent Progress on Optical Micro/Nanomanipulations: Structured Forces, Structured Particles, and Synergetic Applications.

Optical manipulation has achieved great success in the fields of biology, micro/nano robotics and physical sciences in the past few decades. To date, the optical manipulation is still witnessing substantial progress powered by the growing accessibility of the complex light field, advanced nanofabrication and developed understandings of light-matter interactions. In this perspective, we highlight recent advancements of optical micro/nanomanipulations in cutting-edge applications, which can be fostered by structured optical forces enabled with diverse auxiliary multiphysical field/forces and structured particles. We conclude with our vision of ongoing and futuristic directions, including heat-avoided and heat-utilized manipulation, nonlinearity-mediated trapping and manipulation, metasurface/two-dimensional material based optical manipulation, as well as interface-based optical manipulation.

Non-Ultrawide Bandgap Semiconductor GaSe Nanobelts for Sensitive Deep Ultraviolet Light Photodetector Application.

In this paper, the authors report the fabrication of a sensitive deep ultraviolet (DUV) photodetector by using an individual GaSe nanobelt with a thickness of 52.1 nm, which presents the highest photoresponse at 265 nm illumination with a responsivity and photoconductive gain of about 663 A W-1 and 3103 at a 3 V bias, respectively, comparable to or even better than other reported devices based on conventional wide bandgap semiconductors. According to the simulation, this photoelectric property is associated with the wavelength-dependent absorption coefficient of the GaSe crystal, for which incident light with shorter wavelengths will be absorbed near the surface, while light with longer wavelengths will have a larger penetration depth, leading to a blueshift of the absorption edge with decreasing thickness. Further finite element method (FEM) simulation reveals that the relatively thin GaSe nanobelt exhibits an enhanced transversal standing wave pattern compared to its thicker counterpart at a wavelength of 265 nm, leading to an enhanced light-matter interaction and thereby more efficient photocurrent generation. The device can also function as an effective image sensor with acceptable spatial resolution. This work will shed light on the facile fabrication of a high-performance DUV photodetector from non-ultrawide bandgap semiconductors.

Nanostructured multilayer hyperbolic metamaterials for high efficiency and selective solar absorption.

Highly efficient solar-to-thermal conversion is desired for the renewable energy technologies, such as solar thermo-photovoltaics and solar thermo-electric systems. In order to maximize the energy conversion efficiency, solar-selective absorbers are essential with its absorption characteristics specially tailored for solar applications. Here, we propose a wideband spectral-selective absorber based on three-dimensional (3D) nanostructured hyperbolic metamaterial (HMM), which can realize near-unity absorption across the UV and NIR spectral ranges. Moreover, the optical topological transition (OTT) of iso-frequency surface (IFS) is manipulated to selectively enhance light absorption in the entire solar spectrum, crucial for improved energy utilization. Impressive solar-to-thermal conversion efficiency of 95.5% has been achieved. Particularly, such superior properties can be retained well even over a wide range of incident angles. These findings open new avenues for designing high-performance solar thermal devices, especially in the fields related to solar energy harvesting.

Strong hyperbolic-magnetic polaritons coupling in an hBN/Ag-grating heterostructure.

Strong coupling between hyperbolic phonon-polaritons (HP) and magnetic polaritons (MP) is theoretically studied in a hexagonal boron nitride (hBN) covered deep silver grating structure. It is found that MP in grating trenches strongly interacts with HP in an anisotropic hBN thin film, leading to a large Rabi splitting with near-perfect dual band light absorption. Numerical results indicate that MP-HP coupling can be tuned by geometric parameters of the structure. More intriguingly, the resonantly enhanced fields for two branches of the hybrid mode demonstrate unusually different field patterns. One exhibits a volume-confined Zigzag propagation pattern in the hBN film, while the other shows a field-localization near the grating corners. Furthermore, resonance frequencies of these strongly coupled modes are very robust over a wide-angle range. The angle-insensitive strong interaction of hyperbolic-magnetic polaritons with dual band intense light absorption in this hybrid system offers a new paradigm for the development of various optical detecting, sensing and thermal emitting devices.

Strong coupling of optical interface modes in a 1D topological photonic crystal heterostructure/Ag hybrid system.

We theoretically investigate the strong coupling of a topological photonic state (TPS) and Tamm plasmon polaritons (TPPs) in a graphene embedded one-dimensional topological photonic crystal (TPC)/Ag structure in visible range. It is shown that the strong interaction of a TPS at the TPC heterointerface and TPP at the Ag surface enables a large Rabi splitting up to 96.8 meV with a dual-narrow-band perfect absorption. A spectral linewidth of the hybrid mode can be 0.3 nm with a Q factor of 1078. The numerical results also reveal that mode coupling can be either tuned by adjusting the geometric parameters or actively controlled by the incident angle, offering a remarkable polarization-independent strong light-matter interaction. The coupled mode theory is employed to explain the strong TPS-TPP coupling. The polarization-independent and controllable strong mode coupling with a dual-narrow-band perfect absorption in this simple lamellar geometry offers new possibilities for developing various on-chip optical detection, sensing, filtering, and light-emitting devices.

Light Confinement Effect Induced Highly Sensitive, Self-Driven Near-Infrared Photodetector and Image Sensor Based on Multilayer PdSe2 /Pyramid Si Heterojunction.

In this study, a highly sensitive and self-driven near-infrared (NIR) light photodetector based on PdSe2 /pyramid Si heterojunction arrays, which are fabricated through simple selenization of predeposited Pd nanofilm on black Si, is demonstrated. The as-fabricated hybrid device exhibits excellent photoresponse performance in terms of a large on/off ratio of 1.6 × 105 , a responsivity of 456 mA W-1 , and a high specific detectivity of up to 9.97 × 1013 Jones under 980 nm illumination at zero bias. Such a relatively high sensitivity can be ascribed to the light trapping effect of the pyramid microstructure, which is confirmed by numerical modeling based on finite-difference time domain. On the other hand, thanks to the broad optical absorption properties of PdSe2 , the as-fabricated device also exhibits obvious sensitivity to other NIR illuminations with wavelengths of 1300, 1550, and 1650 nm, which is beyond the photoresponse range of Si-based devices. It is also found that the PdSe2 /pyramid Si heterojunction device can also function as an NIR light sensor, which can readily record both "tree" and "house" images produced by 980 and 1300 nm illumination, respectively.

Angle-independent strong coupling between plasmonic magnetic resonances and excitons in monolayer WS2.

The room-temperature strong coupling between plasmonic magnetic resonances (MRs) of metal gratings and excitons in monolayer WS2 is intensively investigated. Both numerical simulations and theoretical calculations indicate that the strong coupling between MRs and excitons enables the remarkable spectral splitting. The typical anticrossing behavior with the Rabi splitting up to 86.5 meV is realized on the color-coded absorption spectra by changing the nanogroove depth, width, and the refractive index of the dielectric filled into nanogrooves, respectively. Interestingly, such strong coupling can also be achieved by using WS2 ribbons instead of the monolayer and simultaneously is dynamically controlled by varying the interaction area. More importantly, the observed MR-exciton coupling is angle-independent. Our findings thus suggest a possible way toward enhancing light-matter interactions in monolayer transition-metal dichalcogenides and play significant roles in quantum and nonlinear nanophotonic devices at ambient conditions.

Strong longitudinal coupling of Tamm plasmon polaritons in graphene/DBR/Ag hybrid structure.

In this paper, strong longitudinal coupling of the Tamm plasmon polaritons (TPPs) is investigated in a graphene/DBR/Ag slab hybrid system. It is found that TPPs can be excited at both the top graphene and the bottom silver slab interface, which can strongly interact with each other in this coupled structure. Numerical simulation results demonstrate that the vertical Tamm plasmon coupling can be either tuned by adjusting the geometric parameters or actively controlled by the Fermi energy in graphene sheet as well as the incident angle of light, allowing for strong light-matter interaction with a tunable dual-band perfect absorption. Moreover, the coupling strength of the hybrid modes exhibits a large tuning range, from a large Rabi splitting to an extremely narrow induced transparency in this coupled regime. Coupled mode theory has been employed to explain the strong coupling phenomenon. The controllable TPP coupling with an ultrahigh dual-band absorption capability offered by this simple layered structure opens new avenues for developing a broad range of graphene-based active optoelectronic and polaritonic devices.

Dual-plasmonic Au/graphene/Au-enhanced ultrafast, broadband, self-driven silicon Schottky photodetector.

High-performance photodetectors are desirable for various applications, including multi-wavelength image sensing, communication, and safety monitoring. In this study, we report the construction of a dual-surface plasmon-enhanced silicon Schottky photodetector using Au nanoparticles (NPs)/graphene/Au NPs hybrid structure as the electrode. It was found that the as-assembled device exhibited broad sensitivity, ranging from ultraviolet to near-infrared light (360-1330 nm) at room temperature, with a high response speed of 360 ns and a 3 dB bandwidth of 780 kHz at zero bias. Further theoretical simulation based on the finite-element method revealed that good device performance is associated with the contribution of the Au NPs/graphene/Au NPs electrode: intense dual-plasmonic resonance coupling is induced in a hybrid structure of two layers of metallic NPs separated by a uniform monolayer graphene. It not only can enhance light trapping and the localized electric field at the resonant and off-resonant wavelength regions, but is also beneficial for the tunneling of hot electrons. This work demonstrated the great potential of dual-plasmonic resonance coupling in optoelectronic devices and will lead to the development of advanced plasmonic devices.

Numerical study on supercontinuum generation by different optical modes in AsSe2-As2S5 chalcogenide microstructured fiber.

We investigate supercontinuum generation (SCG) in AsSe2-As2S5 chalcogenide microstructured optical fibers (MOFs) pumped by different optical modes. The influence on SCG by different optical modes including the fundamental and high-order modes is analyzed numerically. The evolution of the supercontinuum (SC) is investigated by changing the pump wavelength (2120, 2580, and 3280 nm) and peak power (from 200 to 1000 W) of each optical mode (LP01,LP11,LP31) in the MOFs with different fiber lengths. SCG in MOFs with different core diameters is also simulated. The different optical modes cause the variation of the chromatic dispersion profile and the effective nonlinearity, which induces different mechanisms of the SCG and changes the spectral range. The maximum SC spectral range covers 12.931 µm from 1.389 to 14.320 µm when pumped by the LP11 mode with the peak power of 1000 W at 3280 nm. The simulated results will be instructive for the experimental SCG up to the midinfrared waveband longer than 10 µm.

Mesoporous anodic α-Fe2O3 interferometer for organic vapor sensing application.

In this work, we reported the utilization of mesoporous α-Fe2O3 films as optical sensors for detecting organic vapors. The mesoporous α-Fe2O3 thin films, which exhibited obvious Fabry-Perot interference fringes in the reflectance spectrum, were successfully fabricated through electrochemical anodization of Fe foils. Through monitoring the optical thickness of the interference fringes, three typical organic species with different vapor pressures and polarities (hexane, acetone and isopropanol) were applied as probes to evaluate the sensitivity of the α-Fe2O3 based interferometric sensor. The experiment results showed that the as-synthesized mesoporous α-Fe2O3 interferometer displayed high reversibility and stability for the three organic vapors, and were especially sensitive to isopropanol, with a detection limit of about 65 ppmv. Moreover, the photocatalytic properties of α-Fe2O3 under visible light are beneficial for degradation of dodecane vapor residues in the nano-pores and refreshment of the sensor, demonstrating good self-cleaning properties of the α-Fe2O3-based interferometric sensor.

Theoretical investigation on mid-infrared cascaded Raman fiber laser based on tellurite fiber.

A numerical simulation of third-order cascaded Raman fiber laser based on tellurite fiber at the 2-5 µm waveband is presented. The Raman fiber laser can be optimized with the most suitable tellurite fiber length of 0.5-1.0 m and the most reasonable reflectivity of the third-order Stokes output FBG32 of 10%-20%. We demonstrate numerically that the third-order Stokes wave can reach the maximum average power of 45.2 W and the maximum optical conversion efficiency of 45.2%, corresponding to the FBG32 reflectivity of 10% and the tellurite fiber length of 0.3 m with the attenuation of 0.85 dB/m, when pumped by 2 µm light with the average power of 100 W. Our simulated results provide valuable theoretical guidance for the design and experiment of tellurite Raman fiber laser at a mid-infrared waveband.

Total absorption of light in monolayer transition-metal dichalcogenides by critical coupling.

Transition-metal dichalcogenides with exceptional electrical and optical properties have emerged as a new platform for atomic-scale optoelectronic devices. However, the poor optical absorption resists their potential applications. The novel method of critical coupling with guided resonances is proposed to realize total absorption of light in monolayer MoS2 both theoretically and numerically. Simulated results illustrate that the perfect absorption with critical coupling is achieved by choosing suitably the ration of the hole radius to the period of the photonic crystal slab, and that the tunability of absorption peaks is obtained by a small change in the period and the thickness of the slab. Intriguingly, such device manifests the unusual polarization-insensitive feature and the good absorption stability over a wide angle range of incidence. The total absorption in monolayer MoSe2, WS2, and WSe2 is realized handily by the same principle. Hence, our results may open up new possibilities for improving the light-matter interaction in monolayer transition-metal dichalcogenides and find utility in wavelength-selective photoluminescence and photodetection.

Experimental investigation on supercontinuum generation by single, dual, and triple wavelength pumping in a silica photonic crystal fiber.

We investigate the supercontinuum (SC) generation in an 1 cm long silica photonic crystal fiber (PCF) pumped by the pulse sources with single, dual, and triple wavelengths, respectively. The silica PCF has two zero-dispersion wavelengths at 900 and 2620 nm, respectively. When pumped by a single wavelength, the SC spectral range covers about 1000 nm. When pumped by dual and triple wavelengths, the SC spectral range covers wider than 2000 nm. Both the SC spectral range and the flatness are improved obviously when pumped by triple wavelengths. The maximum SC spectral range is obtained when the silica PCF is pumped by the triple wavelengths at 800, 1450, and 1785 nm. The SC spectral range covers 2810 nm from 350 to 3160 nm wider than three octaves. The 10 dB bandwidth covers 2280 nm from 450 to 2730 nm wider than two octaves. This is the first investigation on comparison of the SCs generated by different pump wavelengths up to three experimentally. The generated SC spectra have covered the full transmission window of silica fiber.

Comparative research for the dietary pattern of patients with esophageal cancer at different developing stages and the daily intake of vitamin A, E and ß-carotene.

This paper discusses the different stages of normal esophageal's developing to esophageal cancer, and the difference among dietary patterns of patients with esophageal cancer and acceptable daily intake of vitamin A, E and beta carotene intake in diet. This paper takes advantage of food composition table, calculates the intake amount of dietary vitamin A, E and beta carotene in all kinds of food for patients with esophageal cancer, and analyzes the intake amount difference of dietary vitamin A, E and beta carotene in each kind of food for different groups of people. Research conclusions: the low content level of dietary vitamin A, E beta-carotene and low intake amount of beans, vegetables and fruit intake may increase the risk of esophageal cancer' occurring, while the relationship among dietary vitamin E, the occurrence and development of esophageal cancer needs further discussion.